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In terms of performance (grip) and not the looks these would be my recommendations:
1. 17" and 18" combo over 18" and 19". Tire width? You want the widest and softest tires (lower the treadwear rating, the better) you can fit and still bring them to the operating temp. Tires that are wide and hard, will perform worse than soft narrow tires that are operating its ideal temp range. In 4C the front end is very light, so anything wider than 225 at the front, you will be having hard time to heat up. The rear end is quite heavy though and also has the drive, so you can easily run 265 tires and you'll still heat them up. In my case 215 front and 265 rear seems to be close to the ideal combo. Both tires heat up evenly and wear out pretty evenly as well. I believe that 215 / 275 combo might be even better, but 275 rears are hard to come by. For 215 you need at least 7" wheel width and 9" for 265. Ideally +0.5" up on the minimum wheel width to provide more stability to the tire side wall. Of course, you don't want low profile tires as they poorly absorb road imperfections, temperatures fluctuate a lot and generally drive worse than slightly higher sidewall tires. They look cool though.
2. The rims width should be adjusted to suit the tires and not the other way around. So once you know what tires you will be running, you can choose the optimal wheels width.
3. Alignment. There is no ideal alignment that would work best in all circumstances, but here are some guidelines. Caster is needed to provide straight line stability and dynamic camber gain upon cornering. On a 4C you want as much caster as you can get as the car is already very twitchy. Negative camber is needed to compensate for the body roll and softer your car is sprung and stickier the tires you run, the more negative camber you'll need. With toe you can make car's front or rear end more or less prone to steer. If you want more initial turn in, you'll toe out the front, and if you want more straight line stability and less responsive front end you'll add some toe in at front. However, toe in in the world of performance driving is not a common thing to see. 4C is already very nimble at front, so I would suggest to keep the front toe close to 0°, perhaps a slight toe out on a tight twisted tracks, but no excessive toe out is needed as with FWD or some other nose heavy cars is. On the rear you want a healthy amount of toe in to keep the rear end planted. 4C has very short wheelbase and very wide track, which means a generally nervous car with quick wheel load transfer, so any oversteer that might happen, will happen suddenly and quickly and you definitely don't want a zero toe or even toe out int that situation. Also with all the weight at the rear axle, you can easily reduce the potential understeer with slight throttle lift off and the rear end will start to turn in nicely. Do that with not enough toe in at the rear and you'll drive backwards sooner than you'll realize. This is very simplified, but you get the idea. It is impossible though to say what's the perfect alignment for 4C, without knowing all the details (tires, suspensions, weight, intentions of use, etc.). But let's say you have a mildly modded 4C (better, wider tires, remap, perhaps suspension) and like to occasionally push it, but otherwise you drive normal. In that case, I would recommend about +4°00' of caster, -2°00 deg of front camber, +0°02' of front toe, -2°15' of rear camber and +0°18' of rear toe (with uniballs or uprated control arms, otherwise +0°20'). This will provide a nicely balanced alignment that will be OK for street driving, yet decently perform on a track and won't chew the tires excessively. That's about the performance driving.
1. 17" and 18" combo over 18" and 19". Tire width? You want the widest and softest tires (lower the treadwear rating, the better) you can fit and still bring them to the operating temp. Tires that are wide and hard, will perform worse than soft narrow tires that are operating its ideal temp range. In 4C the front end is very light, so anything wider than 225 at the front, you will be having hard time to heat up. The rear end is quite heavy though and also has the drive, so you can easily run 265 tires and you'll still heat them up. In my case 215 front and 265 rear seems to be close to the ideal combo. Both tires heat up evenly and wear out pretty evenly as well. I believe that 215 / 275 combo might be even better, but 275 rears are hard to come by. For 215 you need at least 7" wheel width and 9" for 265. Ideally +0.5" up on the minimum wheel width to provide more stability to the tire side wall. Of course, you don't want low profile tires as they poorly absorb road imperfections, temperatures fluctuate a lot and generally drive worse than slightly higher sidewall tires. They look cool though.
2. The rims width should be adjusted to suit the tires and not the other way around. So once you know what tires you will be running, you can choose the optimal wheels width.
3. Alignment. There is no ideal alignment that would work best in all circumstances, but here are some guidelines. Caster is needed to provide straight line stability and dynamic camber gain upon cornering. On a 4C you want as much caster as you can get as the car is already very twitchy. Negative camber is needed to compensate for the body roll and softer your car is sprung and stickier the tires you run, the more negative camber you'll need. With toe you can make car's front or rear end more or less prone to steer. If you want more initial turn in, you'll toe out the front, and if you want more straight line stability and less responsive front end you'll add some toe in at front. However, toe in in the world of performance driving is not a common thing to see. 4C is already very nimble at front, so I would suggest to keep the front toe close to 0°, perhaps a slight toe out on a tight twisted tracks, but no excessive toe out is needed as with FWD or some other nose heavy cars is. On the rear you want a healthy amount of toe in to keep the rear end planted. 4C has very short wheelbase and very wide track, which means a generally nervous car with quick wheel load transfer, so any oversteer that might happen, will happen suddenly and quickly and you definitely don't want a zero toe or even toe out int that situation. Also with all the weight at the rear axle, you can easily reduce the potential understeer with slight throttle lift off and the rear end will start to turn in nicely. Do that with not enough toe in at the rear and you'll drive backwards sooner than you'll realize. This is very simplified, but you get the idea. It is impossible though to say what's the perfect alignment for 4C, without knowing all the details (tires, suspensions, weight, intentions of use, etc.). But let's say you have a mildly modded 4C (better, wider tires, remap, perhaps suspension) and like to occasionally push it, but otherwise you drive normal. In that case, I would recommend about +4°00' of caster, -2°00 deg of front camber, +0°02' of front toe, -2°15' of rear camber and +0°18' of rear toe (with uniballs or uprated control arms, otherwise +0°20'). This will provide a nicely balanced alignment that will be OK for street driving, yet decently perform on a track and won't chew the tires excessively. That's about the performance driving.